April 2014
Volume 55, Issue 13
Free
ARVO Annual Meeting Abstract  |   April 2014
The third generation of antihistamines: Assessment of Histamine H1/H4 Receptor Antagonists in a Murine Model of Allergic Conjunctivitis
Author Affiliations & Notes
  • Matt J Chapin
    ORA, Andover, MA
  • Laura Belen
    ORA, Andover, MA
  • Andy Whitlock
    ORA, Andover, MA
  • Jac Wijkmans
    Griffin Discoveries BV, Amsterdam, Netherlands
  • Tiffany van de Meer
    Griffin Discoveries BV, Amsterdam, Netherlands
  • Mounir Andaloussi
    Griffin Discoveries BV, Amsterdam, Netherlands
  • Rogier A Smits
    Griffin Discoveries BV, Amsterdam, Netherlands
  • Iwan de Esch
    Griffin Discoveries BV, Amsterdam, Netherlands
    Medicinal Chemistry, Faculty of Exact Sciences, VU University Amsterdam, Amsterdam, Netherlands
  • Rob Leurs
    Griffin Discoveries BV, Amsterdam, Netherlands
    Medicinal Chemistry, Faculty of Exact Sciences, VU University Amsterdam, Amsterdam, Netherlands
  • Footnotes
    Commercial Relationships Matt Chapin, Ora, Inc (E); Laura Belen, Ora, Inc (E); Andy Whitlock, Ora, Inc (E); Jac Wijkmans, Griffin Discoveries BV (E), Griffin Discoveries BV (P); Tiffany van de Meer, Griffin Discoveries BV (E), Griffin Discoveries BV (P); Mounir Andaloussi, Griffin Discoveries BV (E), Griffin Discoveries BV (P); Rogier Smits, Griffin Discoveries BV (I), Griffin Discoveries BV (P); Iwan de Esch, Griffin Discoveries BV (I), Griffin Discoveries BV (P); Rob Leurs, Griffin Discoveries BV (I), Griffin Discoveries BV (P)
  • Footnotes
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Investigative Ophthalmology & Visual Science April 2014, Vol.55, 2482. doi:
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      Matt J Chapin, Laura Belen, Andy Whitlock, Jac Wijkmans, Tiffany van de Meer, Mounir Andaloussi, Rogier A Smits, Iwan de Esch, Rob Leurs; The third generation of antihistamines: Assessment of Histamine H1/H4 Receptor Antagonists in a Murine Model of Allergic Conjunctivitis. Invest. Ophthalmol. Vis. Sci. 2014;55(13):2482.

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      © ARVO (1962-2015); The Authors (2016-present)

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Abstract

Purpose: This study tested the hypothesis that drugs antagonizing both the H1 and the H4 histamine receptors (H1R and H4R) may provide superior relief for the signs and symptoms of allergic conjunctivitis when compared to traditional allergy therapies.

Methods: The study employed a murine conjunctival allergen challenge (CAC) model to test two structurally unrelated dual-action H1R/H4R antagonists: GD134 and GD136, as well as selective H4R antagonist GD135. Two positive comparators (olopatadine and prednisolone) and a vehicle control were also tested. Test articles were masked to investigators for the duration of the study. Animals (female balb/c mice) were sensitized by injection with a short ragweed allergen (SRW)/adjuvant mixture, and then challenged with topical SRW 17 days later to confirm an allergic response. Nine animals were randomly assigned to each of the 6 treatment groups. Animals received topical applications of test agent on 3 consecutive days, and then underwent CAC twice daily for 4 successive days; test agents were also applied on these days. Mean group values for hyperemia and squinting were compared with vehicle and with baseline to determine test agent effects.

Results: Positive comparators reduced post-CAC hyperemia scores relative to the vehicle controls; these reductions were significant for prednisolone at challenge 1, 4, 6 and 8 (p <0.05). Both H1R/H4R antagonists reduced hyperemia significantly (GD136, 3 of 4 challenges significant at p<0.05; GD134, 4 challenges significantly lower at p<0.05). Selective H4R antagonist GD135 did not significantly reduce hyperemia. Squinting scores exhibited a progressive decline with each successive challenge, however only the scores for olopatadine at challenge 8 were significantly reduced when compared to controls (p<0.05).

Conclusions: Current antihistamine therapy for allergic conjunctivitis focuses on antagonism of the H1R signaling pathway. Despite this, recent studies have revealed not only a role for H4 receptors in the etiology of itch, the hallmark symptom of ocular allergy, but also identified the H4R as a new target to treat inflammation. Our studies provide evidence that two of our test compounds, GD134 and GD136, may have potential efficacy in the treatment of allergic conjunctivitis. Future studies, such as dose-ranging trials or studies in humans will help to clarify their potential.

Keywords: 475 conjunctivitis • 555 immunomodulation/immunoregulation • 557 inflammation  
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