June 2021
Volume 62, Issue 8
Open Access
ARVO Annual Meeting Abstract  |   June 2021
A Spectroscopic Approach to Measuring Meibum Lipid Composition and Conformation in Donors with Sjogren’s Syndrome
Author Affiliations & Notes
  • Sravya Rao Veligandla
    University of Louisville School of Medicine, Louisville, Kentucky, United States
  • Anthony Ewurum
    Chemistry, University of Louisville, Louisville, Kentucky, United States
  • Jordan Swindel
    University of Louisville School of Medicine, Louisville, Kentucky, United States
  • Dr. Jeremy Clark
    University of Louisville School of Medicine, Louisville, Kentucky, United States
  • Douglas Borchman
    University of Louisville School of Medicine, Louisville, Kentucky, United States
  • Footnotes
    Commercial Relationships   Sravya Veligandla, None; Anthony Ewurum, None; Jordan Swindel, None; Dr. Jeremy Clark, None; Douglas Borchman, None
  • Footnotes
    Support  R01 EY026180/EY/NEI NIH HHS/United States; Research to Prevent Blindness, Inc New York, NY, USA GN151619B
Investigative Ophthalmology & Visual Science June 2021, Vol.62, 686. doi:
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      Sravya Rao Veligandla, Anthony Ewurum, Jordan Swindel, Dr. Jeremy Clark, Douglas Borchman; A Spectroscopic Approach to Measuring Meibum Lipid Composition and Conformation in Donors with Sjogren’s Syndrome. Invest. Ophthalmol. Vis. Sci. 2021;62(8):686.

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      © ARVO (1962-2015); The Authors (2016-present)

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Abstract

Purpose : Sjogren's syndrome (SS) is a chronic autoimmune rheumatic disease affecting 3 million individuals in the United States. About 80 % of people with SS have dry eye, keratoconjunctivitis sicca. We measured the composition and conformation of meibum in donors with SS and donors without SS or dry eye since meibum lipid has been associated with dry eye and meibomian gland dysfunction.

Methods : Meibum was collected using an ILUX instrument (Alcon, Fort Worth, TX). Infrared spectroscopy was used to measure meibum lipid conformation (structure). 1H-NMR spectroscopy was used to measure meibum composition.

Results : Meibum was collected from 35 donors without dry eye (Mn) and without SS and eight donors with dry eye and with SS (Mss). The cholesterylester/wax ester ratio was significantly, P = 0.003. higher for Mss 0.51 ± 0.02 compared with Mss, 0.70 ± 0.06. Mss contained significantly, P = 0.02, more straight chains, 67 ± 5 %, compared with Mn, 57 ± 1 %. No statistical difference was apparent, P > 0.05, between the Anteiso Branched, 20 ± 1, 15 ± 1 or Iso Branched chains 23 ± 1, 19 ± 4 of Mn or Mss, respectively. There was no statistical difference, P > 0.05, between the eight phase transition parameters measured for Mss or Mn.: Transition Temperature ( oC), Mn : 30.3 ± 0.4, Mss: 29.9 ± 0.9; Cooperativity, Mn : 7.9 ± 0.4, Mss: 7.6 ± 0.6; Order 36.0 oC (% trans), Mn : 35 ± 1, Mss: 38.4 ± 3.6; Order 33.4 oC (% trans), Mn : 40 ± 1, Mss: 43.3 ± 3.7; Δ enthalpy (kcal/mol), Mn : 142 ± 6, Mss :135 ± 25; Δ entropy (kcal.mol/degree), Mn : 0.48 ± 0.02, Mss: 0.45 ± 0.03; Minimum Frequency (cm-1), Mn : 2849.71 ± 0.06, Mss: 2849.5 ± 0.1; Maximum Frequency (cm-1), Mn : 2853.69 ± 0.09, Mss: 2853.3 ± 0.1.

Conclusions : Inspite of having a higher cholesterylester/wax ester ratio and more straight chains, the compositional differences between Mss and Mn did not affect their phase transition parameters. A higher CE/WE ratio and straight chain composition of Mss compared with Mn, could be a marker for SS and/or contribute to dry eye in patients with SS. Studies are planned to measure the rheology of Mss to test this idea.

This is a 2021 ARVO Annual Meeting abstract.

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